I know I had mentioned it earlier but; Have you tested brand new mixed up water yet?
I use I/O regularly and typically it's Alk is lower than the values shown on the graph that Brian posted and lower than the values in your tank. Certainly it is possible that your alk is that high because of the salt you are using but until you test, you are guessing.
I have spent a lot of time trying to fix something by doing water changes only to find out it was the new saltwater causing the problem. The thread about mixing up saltwater has some good information on this subject.
If your ALK is higher than you want it, I don't think trying to do something to the tank to lower it is the best or safest idea. First & foremost, determine where your getting this high value from, then start working on correcting it. For example, as Brian suggested, if your I/O has excessively high ALk when you mix it up, use another brand or get another bag that mixes closer to where you want it, then start doing water changes to adjust ti where you want it to be. (again in this process you need to test your brand new water to determine that is has the values you are wanting)
Did you (or Nikki) check your mag? It is typically low with I/O as well.
Bringing your ca up is simple but take it slow. You easily could bring it up in just a few minutes but I don't suggest it. Small daily doses until you've reached your goal is safer. It's always easier to add a little more than deal with it being to high and much less stressful on your tank inhabitants. Using the Calcium only part of C-balance is fine and should not cause any additional ALK or PH issues. It is highly likley that your elevated PH is being caused by your higher alk level, they are not the same but Alk does influance your ph. I believe that slightly lowering your alk will also adjust your PH. Don't try to fix both at the same time. Just test daily to see where everything is and in time you will learn what, how much and how often you need to add trace elements to keep your tank where you want it.
Joel